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Using Clang and the LLVM toolchain system wide in Gentoo is experimental. It's been possible to use the toolchain for many years, however there isn't a lot of in depth information for it. The Gentoo Wiki itself is great for getting started and should be read before trying to tackle the enormous hurdle of using Clang system wide, especially when serving an extra side of rice. Unfortunately, there's a lot of stuff outside the scope of the Gentoo Wiki to cover, such as optimization flags unique to Clang.